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41.
Andreas F. Voegele Christofer S. Tautermann Andreas Hallbrucker Erwin Mayer Klaus R. Liedl 《Icarus》2004,169(1):242-249
Sulfurous acid (H2SO3) has never been characterized or isolated on Earth. This is caused by the unfavorable conditions for H2SO3 within Earth's atmosphere due to the high temperatures, the high water content and the oxidizing environment. Kinetic investigations by means of transition state theory showed that the half-life of H2SO3 at 300 K is 1 day but at 100 K it is increased to 2.7 billion years. Natural conditions to form H2SO3 presumably require cryogenic SO2 or SO2/H2O mixtures and high energy proton irradiation at temperatures around 100 K. Such conditions can be found on the Jupiter moons Io and Europa. Therefore, we calculated IR-spectra of H2SO3 which we compared with Galileo's spectra of Io and Europa. From the available data we surmise that H2SO3 is present on Io and probably but to a smaller extent on Europa. 相似文献
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Reactions producing Al‐rich index minerals in the south‐eastern part of the Lepontine Dome (Central Alps, Switzerland) are investigated using mineral distribution maps, microstructural observations and equilibrium phase diagrams. The apparent staurolite mineral zone boundary corresponds to the paragonite breakdown reaction Pg + Grt + Qtz = Pl + Al2O3 + W. Equilibrium phase diagrams show that most natural metapelites do not contain staurolite or alumosilicates as long as univalent cations are predominantly accommodated in white mica. For a wide range of metapelitic compositions the paragonite breakdown releases sufficient Al for the formation of these minerals. Rare occurrences of staurolite and kyanite, north of the formerly mapped mineral zone boundaries, coexist with paragonite and are restricted to extremely Al‐rich bulk compositions. The stable branch of the kyanite‐forming paragonite breakdown reaction above 660 °C yields an additional mapable isograd. The second set of Al‐releasing reactions is biotite‐producing phengite breakdown. However, these reactions are less suitable to produce well defined reaction isograds in the field as they are more continuous and their progress is strongly dependent on bulk composition. Well developed fibrolite in metapelites does not appear until staurolite starts to breakdown. We conclude that amphibolite facies conditions in the study area were attained by decompression, without substantial heating at low pressures. 相似文献
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In the Bavarian Alps (Germany), west of the Isar River, the abyssal deposits of the Lower Barremian to Upper Campanian Rhenodanubian Group consist of siliciclastic and calcareous turbidites alternating with hemipelagic non-calcareous mudstones. The up to 1500-m-thick succession, deposited in the Penninic Basin to the south of the European Plate, is characterized by a low mean sedimentation rate (c. 25 mm kyr−1) over 60 million years. Palaeocurrents and turbidite facies distribution patterns suggest that sedimentation occurred on a weakly inclined abyssal plain. The highest sedimentation rates (up to 240 mm kyr−1) were associated with the calcareous mud turbidites of the newly defined Röthenbach Subgroup, which includes the Piesenkopf, Kalkgraben and Hällritz formations (Middle Coniacian to Middle Campanian). These calcareous turbidites prograded from the west, and interfinger towards the east with red hemipelagic claystone. A high sea level presumably favoured pelagic carbonate production and accumulation on the shelves and on internal platforms in the western part of the basin, whereas siliciclastic shelves with steep slope angles have bordered the eastern part of the basin, where a dearth of turbidite sedimentation and increased Cretaceous oceanic red beds deposition occurred. In contrast to the eustatically-induced Middle Coniacian to Lower Campanian Cretaceous oceanic red beds (calcareous nannoplankton zones CC14 to CC18), red hemipelagites of Early Cenomanian age (upper part of calcareous nannoplankton zone CC9) and early Late Campanian age (upper part of zone CC21 and zone CC22) are interpreted as the result of regional tectonic activity. 相似文献
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Stable isotopes and trace elements in modern ostracod shells: implications for reconstructing past environments on the Tibetan Plateau,China 总被引:1,自引:0,他引:1
Nicole Börner Bart De Baere Lailah Gifty Akita Roger Francois Klaus Peter Jochum Peter Frenzel Liping Zhu Antje Schwalb 《Journal of Paleolimnology》2017,58(2):191-211
Stable isotopes and trace elements in ostracod shells have been used widely in paleolimnological investigations of past lake hydrochemistry and climate because they provide insights into past water balance and solute evolution of lakes. Regional differences in lake characteristics and species-specific element fractionation, however, do not permit generalization of results from other regions or ostracod species to the southern Tibetan Plateau, in part because most common taxa from the southern Tibetan Plateau are endemic to the area. This study evaluated relations between present-day environmental conditions and the geochemical composition of modern ostracod shells from the southern Tibetan Plateau, to assess the suitability of using shell chemistry to infer hydrological conditions. We studied nine lakes and their catchments, located along a west–east transect in the south-central part of the Tibetan Plateau. Stable oxygen and carbon isotope values and trace element concentrations in recent shells from the four most abundant ostracod species (Leucocytherella sinensis, ?Leucocythere dorsotuberosa, Limnocythere inopinata, Tonnacypris gyirongensis) were measured, together with hydrochemical properties of host waters at the time of sampling. Results revealed significant between-species differences in stable isotope fractionation and trace element incorporation into shell calcite. Stable oxygen and carbon isotope values of ostracod shells were correlated significantly with the stable isotope composition of the respective water body \( \left( {\updelta^{18} {\text{O}}_{{{\text{H}}_{ 2} {\text{O}}}} \,{\text{and }}\updelta^{13} {\text{C}}_{{{\text{H}}_{ 2} {\text{O}}}} } \right) \), reflecting salinity and productivity, respectively. Offsets between δ18Oshell and δ13Cshell and inorganic calcite, the latter representing isotopic equilibrium, suggest shell formation of T. gyirongensis during spring melt. L. sinensis reproduces throughout the monsoon season until September and shows several consecutive generations, and L. inopinata molts to the adult stage after the monsoon season in August/September. The influence of pore water δ13C was displayed by L. inopinata, suggesting shell calcification within the sediment. Mg/Cashell is primarily influenced by water Mg/Ca ratios and salinity and confirms the use of this shell ratio as a proxy for precipitation-evaporation balance and lake level. In addition, Sr/Ca and Ba/Ca can be used to infer changes in salinity, at least in closed-basin lakes with calcite saturation. Observed effects of water Sr/Ca and salinity on Sr/Ca incorporation are biased by the presence of aragonite precipitation in the lakes, which removes bioavailable Sr from the host water, resulting in low Sr/Cashell values. Changes in carbonate mineralogy affect the bioavailability of trace elements, a process that should be considered in paleoclimate reconstructions. Oxygen isotopes and Mg/Cashell ratios were unaffected by water temperature. Positive correlations among Fe/Ca, Mn/Ca and U/Ca in ostracod shells, and their negative correlation with δ13C, which reflects organic matter decay, show the potential to infer changes in redox conditions that can be used to reconstruct past oxygen supply to bottom waters and thus past water-circulation changes within lakes. The intensity of microbial activity, associated with organic matter decomposition, can be inferred from U/Ca ratios in ostracod shells. These findings highlight the value of fossil ostracod records in lake deposits for inferring paleoenvironmental conditions on the southern Tibetan Plateau. 相似文献
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In (semi-)arid regions, available water resources are scarce and groundwater resources are often overused. Therefore, the option to increase available water resources by managed aquifer recharge (MAR) via infiltration of captured surface runoff was investigated for two basins in northern Jordan. This study evaluated the general suitability of catchments to generate sufficient runoff and tried to identify promising sites to harvest and infiltrate the runoff into the aquifer for later recovery. Large sets of available data were used to create regional thematic maps, which were then combined to constraint maps using Boolean logic and to create suitability maps using weighted linear combination. This approach might serve as a blueprint which could be adapted and applied to similar regions. The evaluation showed that non-committed source water availability is the most restricting factor for successful water harvesting in regions with <200 mm/a rainfall. Experiences with existing structures showed that sediment loads of runoff are high. Therefore, the effectiveness of any existing MAR scheme will decrease rapidly to the point where it results in an overall negative impact due to increased evaporation if maintenance is not undertaken. It is recommended to improve system operation and maintenance, as well as monitoring, in order to achieve a better and constant effectiveness of the infiltration activities. 相似文献
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